Ultra-sensitive, room-temperature THz detector using nonlinear parametric upconversion

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15 th Coherent Laser Radar Conference Ultra-sensitive, room-temperature THz detector using nonlinear parametric upconversion M. Jalal Khan Jerry C. Chen Z-L Liau Sumanth Kaushik Ph: 781-981-4169 Ph: 781-981-3728 Ph: 781 981 2242 Ph: 781-981-1067 Email: mjkhan@ll.mit.edu jcchen@ll.mit.edu liau@ll.mit.edu skaushik@ll.mit.edu This work is sponsored by the Office of Secretary of Defense Director of Defense Research and Engineering Quick Reaction Funding, Naval Surface Warfare Center Dahlgren Division Chemical, Biological, and Radiological Defense Division and the United States Air Force under AF Contract #FA8721-05-C-0002. Opinions, interpretations, recommendations and conclusions are those of the authors and are not necessarily endorsed by the United States Government.

Outline Motivation Optical Detection of THz Experiment Results Conversion efficiency enhancements Summary and Future Work MJK - 2

Some Terahertz Applications THz Imaging THz Vibrometry Concealed Weapon Detection Medical Applications Voids in Space Shuttle Foam THz Spectroscopy MJK - 3

State-of-Art THz Direct Detectors Significantly above Quantum Limit THz Receiver Challenges Low-noise (quantum limited) High bandwidth Frequency agile Room Temperature Receiver technology at optical frequencies has significantly better performance MJK - 4

Leveraging IR Technology by Terahertz to Optical Conversion THz Photon THz Optics THz Detector Processing Uncoated Large Inefficient Cryogenic Slow THz Photon THz to Optical Converter IR Optics IR Detector Processing Coated Compact Photon-counting Large bandwidth Room temperature Efficient Leverages mature technology at IR regime to address THz gap MJK - 5

Second-order - χ (2) - Nonlinear Optical Interactions Polarization = χ (1) E + χ (2) E 2 Frequency mixing via non-linear polarization current density Very fast Pump photons are down-converted to signal and idler Efficiency is highly sensitive to phase-matching Detection of optical sideband photon implies presence of THz photon MJK - 6

Optical Detection of THz: Laboratory Implementation THz source: Backward Wave Oscillator (2.5 mw at 700 GHz) Optical Source: 1550 nm, 1 W avg, 10 ns pulses, 200 khz rep rate Commercial telecomm thin film band-edge and band-pass filters Optical Receiver: Geiger-mode Avalanche Photodiode (GM-APD) dark count 20kHz and η ~ 20% MJK - 7

Optical Detection of THz: Geiger-mode Avalanche Photo Diode Experimental Results GM-APD counts number of 1- ns gates with photons in 1 s 200K pulses / 1 s P Idler = K P THz ; Idler attenuated by 69 db to reach noise level Min detectable energy: 3.2e- 19J / 1ns gate NEP THz ~ 4.5 pw/hz 1/2 MJK - 8

Improving Conversion Efficiency using Quasi Phase Matching (QPM) Efficient nonlinear conversion requires phase-matched process Phase-match by reversing polarity of nonlinearity periodically Achieved by bonding orthogonal orientations Phase-matched conversion scales as L 2 MJK - 9

Bulk GaAs Quasi Phase-matching by Diffusion- Bonding Bulk GaAs Diffusion Bonded GaAs Initial Results Top Surface Bottom Surface Pristine GaAs Bond Interface Initially exposed surfaces marred by contact layers; Improved polish quality of top and bottom surfaces Experimented with different contact layers Bond interface is clean Improved Process Top Surface Bond Interface MJK - 10

Efficient Upconversion: Bulk GaAs vs. Diffusion-bonded QPM GaAs Phase-matching is necessary to enhance conversion efficiency DB-GaAs (QPM5, QPM6) show efficiency enhancement > 5 db. QPM4: orientation of bonded crystals was uncertain AR-coated QPM shows additional efficiency ~ 2.5 db Conversion efficiency enhanced in quasi-phase matched MIT Lincoln GaAs Laboratory by 5 db MJK - 11

THz Upconversion Detector Performance Current Performance: NEP ~ 800 fw/hz 1/2 Expect to scale NEP to 40 fw/hz 1/2 in the near future MJK - 12

Summary Demonstrated sensitive optical detection Terahertz at roomtemperature using commercial telecomm components Fabricated quasi-phase matched GaAs crystals using a diffusion bonding process Developed an AR coating for 1550nm radiation that absorbs minimally at THz Demonstrated conversion efficiency enhancements due to QPM AR-coated GaAs crystals THz detector NEP ~ 800 fw/hz 1/2 ; comparable to liquid He cooled bolometer Expect significant improvements using more intense optical pump beam and longer QPM crystals. MJK - 13

BACKUP SLIDES MJK - 14

Terahertz Transmission Properties Material Attenuation at 326 GHz Data for typical sample thickness Loss increases significantly with frequency Atmosphere Attenuation at THz MJK - 15

Optical Detection of THz: Comparison with Theory Experiment Theory 3 db discrepancy between theory and experiment Mode mismatch between optical pump and multimode THz beam Phase mismatch k uncertainty Plane wave estimate used instead of Gaussian beams approximation MJK - 16

Bulk GaAs Quasi Phase-matching by Diffusion- Bonding Bulk GaAs Diffusion Bonded GaAs Fabricated 2 layer, 3 layer and 4 layer diffusion bonded stacks Clean bond interfaces achieved Improved in-house polishing capability AR-coating 2-layer stack MJK - 17

Enhanced Upconversion using Quasi Phase-matched GaAs Demonstrated enhanced conversion efficiency with QPM crystal Upconverted THz signal is generated at chopper frequency Two-layer QPM crystal has ~ 5dB better performance than 4 mm bulk GaAs Two-layer QPM crystal has > 20 db better performance than 8 mm bulk GaAs MJK - 18

Optical Source Development and GaAs Characterization Adaptable, High-power, Pulsed Optical Source Developed a highly adaptable highpower pulsed source; variable rep. rate, pulse width, center frequency SNR ~ 50dB; CW power > 4W; Peak power ~ 25kW GaAs Characterization Terahertz and Optical Frequencies Optical group index, n g = 3.56; loss, α = 0.065 cm -1 Measured transmission spectral scans between 500-700 GHz Estimated THz loss, α = 0.2 cm -1 ; MJK - 19

Optimizing THz-to-Optical Conversion: Ongoing Experiments New THz source: Virginia Diode Amplified Multiplier Chain Near Gaussian spatial mode Spatial mode independent of frequency Testing new QPM crystals Preliminary results indicate that better mode results in an improvement of > 3 db MJK - 20