Diode laser systems for 1.8 to 2.3 µm wavelength range

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Diode laser systems for 1.8 to 2.3 µm wavelength range Márc T. Kelemen 1, Jürgen Gilly 1, Rudolf Moritz 1, Jeanette Schleife 1, Matthias Fatscher 1, Melanie Kaufmann 1, Sandra Ahlert 2, Jens Biesenbach 2, 1 m2k-laser GmbH, Tullastr. 72, D-798 Freiburg, Germany 2 DILAS Diodenlaser GmbH, Galileo-Galilei-Str., D-129 Mainz, Germany ABSTRACT High-power diode lasers in the mid-infrared wavelength range between 1.8µm and 2.3µm have emerged new possibilities either for direct military applications or as efficient pump sources for laser sources in the 2-4µm wavelength range for infrared countermeasures. GaSb based diode lasers are naturally predestinated for this wavelength range and offer clear advantages in comparison to InP based diode lasers in terms of output power and wall-plug efficiency. We will present results on MBE grown (AlGaIn)(AsSb) quantum-well diode laser single emitters with emitter widths between 9µm and 2µm. In addition laser bars with 2% or 3% fill factor have been processed. More than 3% maximum wall-plug efficiency in cw operation for single emitters and laser bars has been reached. Even at 22nm more than 1W have been demonstrated with a 3% fill factor bar. Due to an increasing interest in pulsed operation modes for these mid-infrared lasers, we have investigated single emitters and laser bars at 194nm for different pulse times and duty cycles. More than 9W have been measured at 3A with ns pulse time and 1% duty cycle without COMD for a single emitter. Most applications mentioned before need fiber coupled output power, therefore fiber coupled modules based on single emitters or laser bars have been developed. Single-emitter based modules show 6mW out of a 2µm core fiber with NA=.22 at different wavelengths between 187nm and 194nm. At 22nm an output power of 4mW ex fiber impressively demonstrates the potential of GaSb based diode lasers well beyond wavelengths of 2µm. Combining several laser bars, 2W out of a 6µm core fiber have been established at 187nm. Finally for a 7 bar stack at 187nm we have demonstrated more than 8W at A in qcw mode. Keywords: diode laser arrays, laser bars, GaSb diode laser, mid-infrared laser, infrared countermeasure, pump laser 1. INTRODUCTION High power diode lasers emitting at wavelengths between 18 nm and 23 nm open up a wide range of applications as compact and efficient light sources in the fields of infrared countermeasures (IRCM), pumping of solid state 1-2 and optically pumped semiconductor lasers 3 emitting in the 2-4µm regime, low probability of intercept communication links, and trace gas analysis. Civilian applications exist in the fields of laser surgery 4, medical diagnostics 4 and dermatological treatments 4 as well as direct materials processing such as plastics or aqueous varnish processing. For all these applications output powers in the Multiwatt range, long lifetimes, a low-cost packaging technology and fiber coupling are preferable for practical purposes. GaSb based Quantum Well (QW) diode lasers fabricated using the GaSb based (AlGaIn)(AsSb) materials system are naturally predestined for this wavelength range 6-9 and offer clear advantages in comparison to InP based diode lasers in terms of output power and wall-plug efficiency. In this paper, we will present results on high output power (Al- GaIn)(AsSb) quantum-well diode laser single emitters as well as linear arrays consisting of 19 emitters on a 1cm long bar. The emitting wavelengths are 187nm, 198nm 194nm and 22nm. Based on these single emitters and laser bars, fiber coupled modules and laser stacks will be presented. In the next section a short introduction into the fabrication of GaSb based diode lasers will be given.

2. LASER STRUCTURE AND PACKAGING The laser structure used here was grown on ()-oriented 2-inch n-type GaSb:Te substrates by solid-source molecular beam epitaxy 7-11. The active region consists of three nm wide GaInSb QWs with Ga and In concentrations according to the targeted wavelength. The QWs are separated by 2 nm wide lattice matched Al.3 Ga.7 As.3 Sb.97 barrier layers. We have used a narrow waveguide core with a width of each Al.3 Ga.7 As.3 Sb.97 SC layer of only 12nm. The waveguide core is embedded between 2µm wide lattice matched Al. Ga. As.4 Sb.96 n- and p-doped cladding layers. From these epitaxial layer structures 1µm as well as 9µm wide gain-guided broad-area lasers were fabricated using standard optical lithography in combination with dry etching techniques for lateral patterning, and lift-off metallization for p-contact formation. Backside processing started with substrate thinning followed by the deposition of the n-contact metallization and annealing. The wafers were chipped into single emitters with different resonator lengths (1.-1.mm) and stripe widths (9-2µm). The devices were mounted junction side down either by Indium or AuSn solder on goldcoated copper heat sinks (C-mounts). The rear facets are coated with a highly reflective double-stack of Si and SiO 2 films (> 9% reflectivity) and the front facets are coated by a single layer of SiN (2-% reflectivity). In addition linear broad-area laser arrays with 19 emitters on a 1cm long bar were fabricated. The bars were In- or AuSn soldered epi-side down onto passively or actively cooled gold-coated copper heat sinks. The temperature management has been done by heat exchange with a water-cooled bar holder. Figure 1. Packaged GaSb based high-power broad-area diode lasers. The laser structures have been grown on 2-inch n- type GaSb:Te substrates. 3. SINGLE EMITTER PERFORMANCE Figure 2 shows the output power-vs.-current characteristics and the current dependent wall-plug efficiency of broadarea single emitters at 194nm in cw mode and in pulsed mode (pulse conditions are ns pulse time and 1% d.c.). The resonator length is µm, the stripe width is 2µm. In cw mode at A we have achieved 1.4W. The maximum wallplug efficiency is more than 3% at 1.9A which corresponds to.w output power. Even at A the wallplug efficiency is clearly above 2%. In cw mode the maximum output power is mainly limited by heat and therefore by packaging techniques. To test for COMD effects, for a x2µm 2 single emitter at 194nm the operation current has been ramped up to 3A resulting in 9W. No sudden failure has been detected. The measured far field distribution (1/e 2 definition) in the slow and in the fast axis is shown in figure 3 for a 1 x µm 2 and a 9 x 1 µm 2 single emitter. The slow axis far fields show a strong dependence on the current density due to significant self-heating of the devices as a result of the lower wall-plug efficiency (e.g. in comparison to GaAs based high-power diode lasers) and thus increased heat dissipation. For fiber coupling a smaller stripe width such as 9 µm will be more preferable, but a smaller stripe width is connected with a wider far field typically. In the case of GaSb based diode lasers, heat dissipation plays an important role and therefore by increasing the resonator length to 1 µm it was possible to design a diode laser with a decreased stripe width of 9 µm and the same slow axis far field as a 1 µm wide broad-area diode laser. The fast axis far fields show current independent values of 79 in 1/e 2 definition or 44 FWHM and enable the use of standard optics and efficient coupling to fibres.

The long-term reliability of these diode lasers has been tested by aging some devices at a heat sink temperature of 2 C (figure 4). The batch of four devices has been tested under constant current condition at 3 A. The initial output power is about.9w. All devices show only gradual degradation even after. hours of continuous operation. 1.4 1.2 1..8.6.4.2 λ = 194nm 2xµm 2 T = 2 C, cw. 1 2 3 4 6 lifetime (hours) 3 3 2 2 1 wallplug efficiency (%) 8 6 4 2 λ = 194nm 2xµm 2 pulse conditions: ns, 1% d.c. 1 2 2 3 Figure 2. Output power-vs.-current characteristics and current dependent wall-plug efficiencies of different broad-area single emitters. The measurements have been carried out at a heat sink temperature of 2 C in continuous wave mode (cw) (left hand-side) and in pulsed mode (right hand-side, ns, 1% d.c.). intensity (normalized units) 1. I = 4 A.8.6.4.2. -9-4 4 9 slow axis far field (degree) 2 2 1 T = 2 C, cw 1 x µm 2 9 x 1 µm 2 1 2 3 4 fast axis far field (degree) Figure 3. Slow axis and fast axis far fields of a x 1 µm 2 and a 1 x 9 µm 2 single emitter at 194 nm. 1..9.8 T = 2 C, cw λ = 198nm 1xµm 2.7 2 3 4 6 7 8 9 1 lifetime (hours) Figure 4. CW output power vs. time for a set of 4 emitters. The measurements have been performed at a heat sink temperature of 2 C in cw operation.

4. DIODE LASER ARRAY PERFORMANCE Linear arrays of 19 broad area emitters with a strip width of 1µm (3% fill factor) or 9µm (2% fill factor) and a centre-to-centre spacing between the individual laser strips of µm have been fabricated and In-soldered p-side down on passively and actively cooled heat sinks. The resonator length of the lasers was 1nm to allow for better heat dissipation. Table 1 gives an overview of the electro-optical characteristics of 187nm, 198nm, 194nm and 22nm laser bars shown in figures and 6 both in cw and in pulsed mode. For an actively cooled 198nm laser array with 3% fill factor a maximum output power of 19.W at 68A has been achieved (figure 6). For a passive cooled 187nm laser bar with 2% fill factor in pulsed mode a maximum wallplug efficiency of more than 46% has been measured together with a record slope efficiency of.9 W/A. A maximum cw power of 16 W has been demonstrated at 7A for a 19 emitter array emitting at 22nm (figure ), only limited by thermal rollover and not by a COMD. The saturation of the current-power curve at higher currents is caused by array heating. A high maximum wall-plug efficiency of more than 23% has been measured at 3A for an array emitting at 22nm. This is to our knowledge the highest cw output power and wall-plug efficiency of a diode laser array emitting above 2µm ever reported. The long-term reliability of these laser bars has been tested by aging some devices at a heat sink temperature of 21 C (figure 7). The batch of three bars has been tested under constant current condition at an initial output power of W. After 3 hours laser bars have been controlled by a P-I-U measurement and again started, but this time at 14 W initial output power. Tests are at the moment at 7 hours and are ongoing. emitting wavelength (nm) 187 198 194 22 number of emitters 19 2 19 19 emitter design (µm) 1 x 1 x 9 x 1 1 x fill factor 2% 3% 2% 3% heat sink passive active passive passive Operation mode pulsed cw cw cw heat sink temperature ( C) 2 2 2 17 I th (A) 7.8.1 7. s.e. (W/A).9.28.28.3 η max (%) 46 2 29 23 Table 1. Overview of electro-optical characteristics of different broad-area laser arrays. The data have been measured at a heat sink temperature of 2 C and continuous wave (cw) operation. 2 1 3 2 2 1 λ = 194 nm 2% Fill Factor 2 3 4 6 7 2 1 2 3 4 6 7 λ = 22 nm 3% Fill Factor 3 2 2 1 wallplug efficiency (%) Figure. Output power-vs.-current characteristic of diode laser arrays with 2% and 3% fill factor emitting at 194 nm and mounted on passively cooled heat sinks. The measurements have been carried out at a heat sink temperature of 2 C in CW operation.

2 1 T = 2 C, cw 3 3 2 2 1 λ = 198nm 3% Fill Factor actively cooled 2 3 4 6 7 2 1 4 3 2 λ = 187m 3% Fill Factor 12Hz, 2% d.c. 2 3 4 6 wallplug efficiency (%) Figure 6. CW output power vs. current characteristics recorded for diode laser arrays emitting at 198 nm and 187 nm. 2 1 λ = 194nm 2% fill factor measurement artefact T = 21 C, cw 2 3 4 6 7 8 lifetime (hours) Figure 7. CW output power vs. time for a set of 4 laser bars. The measurements have been performed at a heat sink temperature of 21 C in cw operation.. LASER MODULES AND STACKS The diode laser single emitters and laser arrays are suitable for fiber coupling. In fig. 9 broad-area single emitters with 1xµm 2 design emitting at 193nm and 22nm have been coupled into 2µm core fibers (NA=.22). At 187nm maximum peak power ex fiber was 29mW corresponding to a coupling efficiency of 7%. At lower output powers coupling efficiency is in the range of 8%. For 22nm a maximum peak power ex fiber of 23mW has been demonstrated, corresponding to a coupling efficiency of 8%. Fig. shows the results for fiber coupled laser arrays at 194nm. For a 1-bar module a maximum peak power ex fiber of 7.4W has been established for a 4 µm core fiber (7% coupling efficiency). Taking an 8 µm core fiber 8.7W ex fiber has been demonstrated (8% coupling efficiency. Several laser arrays can be coupled to achieve even higher output powers. For a 3-bar module a peak power of 2W has been measured out of a 6µm core fiber with NA.22. Finally a laser stack has been built consisting of 7x 3% fill factor bars emitting at 187nm (figure 11). In qcw mode (pulse conditions: 2µs pulse time and 12 Hz) a maximum output power of 87W at A has been achieved.

Figure 8. Fiber coupled modules based on GaSb high-power broad-area diode lasers. output power (mw) 8 7 6 4 3 2 FAC + SAC ex fiber λ = 187 nm 1x1 µm 2. 1. 1. 2. 2. 3. 3. 4. 8 7 6 4 3 2 single emitter based modules λ = 22 nm x1 µm 2. 1. 1. 2. 2. 3. 3. 4. Figure 9. CW output power vs. current characteristics for different fiber coupled single emitter based modules emitting at 194nm and 22 nm. All measurements have been performed at 2 C heat sink temperature. output power (mw) 12 8 6 4 FAC + SAC ex fiber (4µm) ex fiber (8µm) λ = 194 nm 1-bar module 2 ex fiber (6µm) 1 λ = 194 nm 3-bar module 2 2 2 3 3 4 4 1 2 2 3 3 4 Figure. CW output power vs. current characteristics for different fiber coupled bar based modules emitting at 194nm. All measurements have been performed at 2 C heat sink temperature.

9 8 7 6 4 3 2 λ = 187nm 7 bar stack T = 2 C, 2µs, 12Hz 2 2 3 3 4 4 operation Figure 11. CW output power vs. current characteristics for a 7-bar-stack at 187nm. All measurements have been performed at 2 C heat sink temperature in pulsed mode with 2µs pulse time and 12Hz. 6. CONCLUSION Recent advances in high-power (AlGaIn)(AsSb) based diode lasers in the 2 µm spectral range have been reported. These diodes are favorable as compact and efficient light sources either for military or civilian applications. High power diode lasers at 187nm, 198nm, 194 nm and 22 nm with 1W of output power have been reported. 2 W in continuous-wave mode at a heat sink temperature of 2 C have been achieved for linear arrays with 19 emitters at 198nm. From a 187nm laser bar measured in pulsed mode more than 46% wallplug efficiency has been demonstrated. These output powers and wallplug efficiencies are among the highest reported so far for GaSb based diode lasers. For a passively cooled laser array at 22nm a wall-plug efficiency of 23% has been reported. This is to our knowledge the highest cw wall-plug efficiency of a diode laser array emitting above 2µm ever reported. Future directions for R&D in the field of high-power (AlGaIn)(AsSb) based laser arrays with respect to reduced prices for (AlGaIn)(AsSb) diode laser arrays is the GaSb substrate size. So far all reported III-Sb based diode lasers have been grown exclusively on 2-inch n-type GaSb:Te substrates. However, to fabricate linear diode laser arrays more costeffectively, the size of the available substrates should be increased to at least 3-inch diameter. 7. ACKNOWLEDGEMENT The authors would like to thank Marilena Herbstritt and Stefan Moritz for excellent technical assistance, Kristin Wieching and Volker Sinhoff from Ingeneric GmbH for valuable contributions. REFERENCES 1. M. Mond, D. Albrecht, E. Heumann, G. Huber, S. Kück, V. Levchenko, V. Yakimovich, V. Shcherbitsky, V. Kisel, N. Kuleshov, M. Rattunde, J. Schmitz, R. Kiefer, J. Wagner, 1.9 µm and 2. µm laser diode pumping of Cr 2+ :ZnSe and Cr 2+ :CdMnTe, Opt. Lett., 27, p. 34, 22 2. B. Rösener, N. Schulz, M. Rattunde, C. Manz, K. Köhler, J. Wagner, High-power, high-brightness operation of a 2.2µm (AlGaIn)(AsSb)-based barrier-pumped vertical-external-cavity surface-emitting laser, IEEE Photon. Technol. Lett. 2, pp. 2, 28. 3. C. Nabors, J. Ochoa, T. Fan, A. Sanchez, H. Choi, G. Turner, Ho:YAG laser pumped by 1.9 µm diode, IEEE J. Quantum Electron. 31, 163, 199

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