Single-frequency operation of a Cr:YAG laser from nm

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Single-frequency operation of a Cr:YAG laser from 1332-1554 nm David Welford and Martin A. Jaspan Paper CThJ1, CLEO/QELS 2000 San Francisco, CA May 11, 2000

Outline Properties of Cr:YAG Cr:YAG laser design considerations Broadband laser results Single frequency design and results Summary

Cr 4+ :YAG energy-level diagram ( D 2d ) 3 A 2 1 E 3 E 1 E 3 E 1 A 1, 1 B 2, 1 A 2 ESA ESA 3 E, 3 A 2 3 B 2 1 A 1, 1 B 1 3 B 1 Pump Laser Non-radiative Complications: Cr 3+ ions Charge-compensation ions Multiple sites Ref: Chang et al, OSA TOPS Vol. 19, ASSL

Cr:YAG emission (not gain) spectrum Eilers et al, IEEE JQE 29, 2508 (1993)

Water-vapor absorption is an issue 100 90 80 6 Torr pressure, 1-m path 70 Absorption (%) 60 50 40 30 20 10 0 1300 1350 1400 1450 1500 1550 1600 Wavelength (nm)

Tetrahedral symmetry for Cr in YAG leads to large transition cross sections, short lifetime Crystal Center wavelength (nm) Tuning range (nm) Eff. gain cross section Lifetime (μs) Max. eff. (10-19 cm2) Ti:sapphire 800 680-1100 2.5-3 3.2 1.0 Cr:LiSAF 850 780-1050 0.32 67 0.53 Cr:YAG 1430 1340-1570 3 4 0.25 Cr:ZnSe 2400 2300-2500 8 7 1.0 Ce:LiSAF 292 280-297 60 0.028 0.35-0.7 Note: we measured 4.5-4.6 microseconds Cr:YAG lifetime at 300 K (radiative QE is likely less than unity, since 4 K lifetime is 25-30 usec)

Cr:YAG absorption spectrum?? 3 E 3 B 2, 3 E, 3 A 2 Pump Eilers et al, IEEE JQE 29, 2508 (1993)

Design considerations for cw Cr:YAG lasers For various reasons, the concentration of Cr 4+ centers is limited, so pump absorption is typically 1 cm -1 This limits pump focusing because of diffraction of pump beam in crystal absorbing region. Favors diffraction-limited pump laser. ESA of pump, bleaching of ground state absorption and thermal quenching call for minimizing pumping levels Both output coupling and cavity losses must be minimized to permit reasonable efficiencies. Gain is limited. Crystal temperature rise must be minimized to avoid increasing the threshold pump level Despite variations in crystal environment for active ion, the broadband nature of the vibronic transition means the laser is essentially homogeneously broadened Elimination of spatial hole burning should lead to singlefrequency operation, similar to Nd:YAG and Ti:sapphire

Pump laser is diode side-pumped Nd:YLF Gain module Nd:YLF slab 1047 nm Diode Laser bar System is early prototype of Q-Peak MPS-1047 CW 10 Available TEM 00 pump power 7 W

Standing-wave, Cr:YAG broadband tuning 1400 1200 Pump: 7.3 W T = 1.75% T = 1.25% Output power (mw) 1000 800 600 400 T = 0.50% 200 0 1340 1380 1420 1460 1500 1540 1580 Wavelength (nm)

Towards tunable, single-frequency operation Basic approach to single-frequency operation was to make a unidirectional, 4-mirror ring cavity, similar to Ti:sapphire ring laser Because of the low gain in Cr:YAG and the need to minimize intracavity losses, the choice of an optical diode is critical. For the non-reciprocal element, we looked at: YIG TGG Various glasses Cr:YAG The best results were obtained by using the gain medium itself as the element. We placed a small magnet near the laser crystal, and aligned the cavity out of plane to compensate for the Faraday rotation

Schematic of Cr:YAG single-frequency laser MPS-1047 CW10 DIODE-PUMPED Nd:YLF LASER OUTPUT CaF 2 ETALON M4 M3 Single-plate birefringent tuner M2 M1 Cr:YAG CRYSTAL (in magnetic field) PUMP LENS 1047-nm PUMP BEAM

Cr:YAG laser layout OC Etalon HR BRF Cr:YAG Pump

Single-frequency tuning curves 800 700 Output power (mw) 600 500 400 300 200 100 Mirror set 1 T=0.5% Mirror set 2 T=0.1% 0 1300 1350 1400 1450 1500 1550 1600 Wavelength (nm)

Scanning Confocal Etalon traces Upper trace: 100x expansion 3.6 MHz linewidth (etalon limit) Lower trace: Two peaks 2 GHz spacing (etalon FSR)

Summary Cr:YAG has some fundamental limits to efficiency and gain because of the ion energy-level structure and interaction with the host crystal Despite these limits, Cr:YAG, when pumped by a diffraction-limited, multi-watt laser, can provide Watt-level cw outputs in a broadly tunable wavelength region centered around 1470 nm Because the laser transition is essentially homogeneously broadened, efficient, single-frequency operation is possible by elimination of spatial hole-burning We obtained single-frequency, broadly tunable (1332-1554 nm) operation (0.68 W max. power) by using the laser crystal itself as the Faraday element in a unidirectional, non-planar ring cavity