Sept 24-30, 2017 LLNL-PRES

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Sept 24-30, 2017 Constantin Haefner, Craig Siders, Andy Bayramian, David Alessi, Kyle Chestnut, Al Erlandson, Eyal Feigenbaum, Tom Galvin, Paul Leisher, Emily Link, Dan Mason, Bill Molander, Paul Rosso, Margareta Rehak, Kathleen Schaffers, Tom Spinka LLNL-PRES-730848 This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. Lawrence Livermore National Security, LLC

The laser: 50 years of discoveries Testimony by Charles Townes The history of the laser is a perfect example of the impact of basic research, not only on science, but also on economy a spectacular impact, often completely unexpected. 2

1996: The First Petawatt Laser, invented at LLNL: 600 J, >1 PW Petawatt achievements and discoveries: 1.3-PW = 1,300,000,000,000,000 Watts ~10 21 W/cm 2 10-100-MeV electron beams Laser made proton beams Hard x-rays and gamma-rays Photo-fission 3

20 years later: HAPLS laser runs 200,000 times faster than the original 1996 Petawatt 4

Worldwide scientific laser facilities mostly meet the demands for proof of principle experiments High-field ICF/IFE/HED Mat.Phys. l 3 Ultrafast Average Power WDM SPL Pumps Industrial Appl. List of lasers indicative and not complete Operational In Build Conceptual 5

Commercial and advanced scientific short pulse laser applications require high repetition rate Neutron Material dev HAPLS Hadron Therapy Neutron Radiography Electron accelerator Max Achievable Intensity Operational In Build Conceptual 6

Heat can be extracted through the edge or the face Rod amplifiers THIN DISK: active mirror multislab-face-cooling Laser emission Pump light Pump light Laser emission Conductive cooling through edges Stress orthogonal to laser beam High energy storage Conductive cooling through back side Stress parallel to laser beam Low energy storage Conductive/convective cooling with liquid (National Energetics) or Helium gas (LLNL, RAL) Stress parallel to laser beam High energy storage 7

LLNL pioneered gas-cooling of high energy laser amplifiers in the eighties: slabs are cooled by rapidly flowing He-gas Gas-cooled amplifier schematic HAPLS production Amplifier Assembly Helium Amplifier slabs Pump Pump Face cooled Nd:Glass slabs Room temperature Helium gas coolant Gas acceleration vanes Mach 0.1 Cooled ASE Edge claddings 8

Two architectures for high energy DPSSL recently demonstrated: the LLNL s HAPLS, and Rutherford s DiPOLE100 Delivers 200J, 20ns, 10Hz and 30J, 1PW, 30fs, 10 Hz Nd:Glass Ti:Sapphire YAG compound ceramics Delivers 100J, 10ns, 10Hz 9

Diode pumping has a significant impact on system efficiencies Ti:Sa PW Efficiency WP 0.4% 2.6% EO 0.6% 3.8% 250J 200J 150J 100J Waste energy per 1J laser output 50J 0J output waste 10

Scale a flashlamp-pumped Ti:Sa laser to TeV-Collider size and you need a nuclear power plant in your backyard. PETRA III 11

HAPLS is designed to deliver Petawatt peak power laser pulses at energy 30J and 10Hz repetition rate = 300 Watt Requirement Specification Energy 0.8 µm 30 J Pulse length 30 fs Peak power 1 PW Pre-pulse power contrast 10-9 c 10-11 Energy stability 0.6% rms Technology DPSSL pumped Ti:sapphire CPA Repetition rate 10 Hz Electrical consumption <150 kw 12

13

HAPLS today.at ELI Beamlines ready for installation 14

Today, the HAPLS delivers 16J of broadband laser pulses at 3.3 Hz; full aperture is pulse duration 28fs NF and FF Profiles at energy (first results, adaptive mirror not active) 500 1000 500 500 1000 1000 500 1000 Full Aperture Pulse duration HAPLS output NF Encircled energy in DL spot = ~0.5 1 hour µ = 28.1 fs σ = 1.4fs = 5.0% 20fs pulse shape Day-to-day optimized 15

HAPLS relies on a diode pumped, indirect chirped pulse amplification architecture ( diode pumped laser pumped laser DPSSL pump lasers Frontend Pulse shaping and contrast enhancement Stretcher wideband Multipass Amplifier Alpha Amplifier Deformable Mirror Modified NIF front-end Pump power amplifier Harmonic converter Beam Conditioning Beta (Power) Amplifier 3.2 MW laser diode arrays Power amplifier diagnostics Compressor Integrated Controls Target ELI Beamlines facility control system 16

The HAPLS Pump laser delivers 1.2 MJ/hour today The HAPLS Petawatt laser system delivers 190 kj/hour Ramped to its full performance at ELI, HAPLS will deliver 1MJ/hr of Petawatt, 30fs pulses

The average power scalability of energetic Ti:Sapphire (and OPCPA) laser is constrained by the availability of pump lasers Indirect CPA: Lamp-pumped SSL pumped Ti:S Waste Output 1-J Efficiency WP EO 0.4% 0.6% Indirect CPA: DPSSL-pumped Ti:S 1-J 2.6% 3.8% -250-200 -150-100 -50 0 Energy [J per J of short-pulse output] Pump trans (~20W) Incident Pump Light (~1kW absorbed) Output beam (~400W) ASE to Cladding Other losses (~80W) (~150W) ASE and quantum defect heat extracted by gas flow Quantum defect heating(~350w) The short gain lifetime and the large quantum defect make Ti:Sapphire drives the cost of the pump laser and makes it an unattractive HAP laser medium 18

The HAPLS pump architecture utilizes dual diode-pumped surface-cooled multislab amplifiers in a 4-pass polarization switched architecture Adaptive optic Adaptive optic l/4 Relay He gas cooling HAP Compressor Ti:sapphire Amplifier Diodes Frequency Injection Converter Transport Long Pulse Front End He gas cooling Relay Relay Polarizer Diodes Diodes Spatial Filter Amp 2 Amp 1 19

The dual diode-pumped surface-cooled multislab amplifier in a 4-pass polarization switched architecture is a template for high average power high peak-power systems Injection Transport High Contrast Short Pulse Front End Relay Relay Adaptive optic l/4 Relay He gas cooling HAP Compressor He gas cooling Polarizer Diodes Diodes Diodes Spatial Filter Amp 2 Amp 1 Example: Scalable High-power Advanced Radiography Capability (SHARC) 20

The HAPLS pump laser could be converted to a 150J, 150fs, 10Hz secondary source driver: SHARC Continuous 1hr run delivering 100Joule pulses at 340W Energy stability scales with output energy. Predicted <0.35% @ 200J Output beam profile 100 Energy (J) 80 60 40 Eave = 100.97 E ave rms =101J = 0.72% de=0.7% RMS 20 0 0 10 20 30 40 50 60 70 Time (mins) 21

Based on HAPLS pump laser and NIF ARC technology, LLNL has developed a concept for a Scalable High-average-power Advance Radiographic Capability (SHARC) SHARC is a low-risk high-trl extension of HAPLS pump laser technology 150J, 150fs, 10Hz, 90/110 db temporal contrast 10-Hz PW (150J/150fs) at greater efficiency than HAPLS (~5% Wall plug efficiency) HAPLS diode-pumped Nd:Glass pump laser with broadband mixed-glass frontend and LLE s Short Pulse OPA seed technology High efficiency, actively cooled MLD-grating laser pulse compressor Application space targets proton-/neutron-particle beam and high brightness x-ray generation 22

Based on HAPLS pump laser and NIF ARC technology, LLNL has developed a concept for a Scalable High-average-power Advance Radiographic Capability (SHARC) Indirect CPA: Lamp-pumped SSL pumped Ti:S Waste Output Efficiency WP EO 0.4% 0.6% 1-J Indirect CPA: DPSSL-pumped Ti:S 2.6% 3.8% 1-J Direct CPA: SHARC 1-J 5.0% 7.2% 23

HAPLS-100 and SHARC could get us to kw to ~10kW of average power (at Petawatt peak power). But we need 100s 9.2017 of LLNL- kw C.Haefner-EACC for 2017 TeV Italy Collider stage. 24

High-Power Single-Aperture Laser Beamline Performances Laser Media Ti:Sa Nd:g HAPLS Yb:X Er:X Cr:X DOE LWFA Roadmap TeV Unit Cell OPA Tm:X Gas Operational In Build Conceptual De-activated Thin Disk Fibers Pulse Energy Pushing the frontiers of high-power applications and high-intensity science requires next-generation high repetition-rate high-energy solid state lasers. 25

Transitioning from Application Space to Laser Media Space If we normalize this plot by the beam area in the final amplifier, the axes become proportional to laser media parameters: photon energy, gain cross-section, gain lifetime, gain bandwidth (ie transform limited pulse duration). PW/cm 2 h kw/cm 2 h 1 gain 26

Power Scaling for Energy-Storage Laser Media (simple scaling w/o architecture considerations) h Laser Media Higher peak power/unit area Ti:Sa Nd:g Yb:X Er:X Cr:X Tm:X Higher average power/unit area Gain Bandwidth h 1 [1] M. D. Perry and G. A. Mourou, Science 264, 917 (1994). gain 27

Stored energy can be extracted from laser medium with a high fluence single pulse, or multiple low-fluence pulses within the radiative lifetime 5 Single-Pulse Extraction 5 Multi-Pulse Extraction 1 1 rad rad Multi-pulse extraction reduces the effective fluence in the laser system and therefore moves the operating point into a manageable regime for low cross-section materials 28

Efficient Diode-Pumped Media for High-Power Lasers (Single-pulse and Multi-Pulse Extraction) h better Laser Media Ti:Sa Nd:g Yb:X Er:X Cr:X Single-Pulse Extraction Multi-Pulse Extraction Optical Damage & B-Integral Limit Tm:X Gain Bandwidth h 1 gain 29

Power Scaling for Energy-Storage Laser Media: Damage Limited Fluence and Multi-Pulse Extraction Min[ h,f dam ] Single-Pulse 5 Extraction 5 Multi-Pulse Extraction Laser Media 1 1 Ti:Sa rad rad Nd:g Yb:X Er:X Cr:X Tm:X Gain Bandwidth h 1 gain 30

Quantum Defect and Gain Lifetime for Energy-Storage Laser Media Laser Media Ti:Sa (1 QD ) conversion diode Media down select for efficient CW Diode Pumping Tm:YLF Nd:g Yb:X Er:X Cr:X Tm:X Ti:S Gain Bandwidth 31

High-Power Single-Aperture Laser Beamline Performances Laser Media Ti:Sa Nd:g Tm:YLF 10-10 10-11 10-9 10-8 Yb:X Er:X Cr:X OPA Tm:X Gas Operational In Build Conceptual Pulse Energy De-activated 33

BAT: Big Aperture Thulium Laser. BAT is a high rep-rate PW-class architecture which scales to 300-kW average power Extension of HAPLS diode-pumped gas-cooled architecture Tm:YLF laser media (1.9um) Commercially available in sizes for 300-kW superior thermal wave front (-dn/dt vs thermal expansion) anisotropic media - de-polarization not an issue Pulse duration 40fs < t < 100fs TL Two-for-one pumping by self-quenching in Tm enables low QD pump scheme True CW pumped: Tm has long lifetime which when combined with the desired pulse repetition rates enables multi-pulse extraction and continuous pumping Quasi-4-level losses are distributed among hundreds of pulses minimizing this effect Efficient extraction at low fluence per pulse, low B, higher efficiency ~40x lower diode cost compared to HAPLS; lower electronics cost due to simplicity over QCW Efficient high-power pump diodes consistent with Tm pumping already on the market We have purchased 300kW-equivalent size Tm:YLF boules, produced our first Il 2 advantage with 1.9um for accelerator applications, eyesafe wavelength regime amplifier slabs and characterizing the material further for its suitability Tm:YLF crystal recently procured by LLNL: Diameter ~10cm 34

Block diagram of BAT Integrated Controls Diode Arrays Front End 3kW (300mJ @ 10kHz) Diode Arrays ~$100k Oscillator Pulse shaping and contrast enhancement Stretcher Multipass Pre-amp Innoslab 3J @ 10kHz minibat amplifier ~750kW cwlaser diode arrays 38J @ 10kHz BAT amplifier BAT Output Sensor 300 kw Compressor Beam transport Target 35

BAT emits 300kW from a single aperture 7cm Characteristic Gain medium Architecture Output energy Repetition rate Average output power Value Tm:YLF Multi-pass, multi-pulse gas cooled 30 J 10,000 Hz 300 kw Wavelength ~ 1.9 µm Output fluence 0.7 J/cm 2 B integral (Poweramp) < 0.1 radians (!!!) 36

BAT laser diodes are always on!!! Commercial pump cw-diode arrays are available (150W/bar) from multiple vendors Power (t) Diode emission Power (t) Diode emission Time [t] Time [t] 2x 808 nm pump band matches Nd:YAG pump wavelengths HAPLS BAT Laser Average Power (kw) 0.3 300 # of arrays 4 4 Array Peak Power (kw) 800 188 Array Average Power (kw) 2.4 188 Emitting area (W x H cm 2 ) 5.6 x 13.4 6.6 x 28.4 Duty Cycle (%) 0.3 100 Relative Cost / array 1 1.9 Diodes for a 300 kw class BAT system are only 1.9X the cost of the HAPLS arrays 37

High-Power Single-Aperture Laser Beamline Performances Laser Media Ti:Sa Nd:g Yb:X Er:X Cr:X OPA Tm:X Gas Operational In Build Conceptual De-activated Pushing the frontiers of high-power applications and high-intensity science requires next-generation high repetition-rate high-energy solid state lasers. 38

High-Power Single-Aperture Laser Beamline Performances Laser Media Ti:Sa 10-10 10-11 10-9 Nd:g 10-8 Yb:X Er:X Cr:X OPA Tm:X Gas Operational In Build Conceptual De-activated Tm Front End (TD/Inn oslab) Tm gascooled mini BAT Laser Tm gascooled BAT Laser Pulse Energy Pushing the frontiers of high-power applications and high-intensity science requires next-generation high repetition-rate high-energy solid state lasers. 39

Summary LLNL is exploring avenues to break the kw barrier for high peak power lasers to drive high flux x- ray, ɣ-ray, and particle beams Performed extensive architecture and material study. Crucially important for high average power lasers is high wall-plug efficiency: reduce heat (once heat is in it s expensive and hard to pull it out) and heat effects (heating-cooling gradients cause beam deterioration, break stuff and limit average power) Direct CPA increases dramatically the efficiency; beam quality and temporal pulse contrast require additional attention Long radiative lifetime gain media become available through multi-pulse extraction at safe energy extraction fluencies CW-pumping reduces massively the capital cost for high average power DPSSL Indirect CPA: Lamp-pumped SSL pumped Ti:S Indirect CPA: DPSSL-pumped Ti:S Waste Output 1-J 1-J Efficiency WP 0.4% 2.6% EO 0.6% 3.8% Direct CPA: SHARC 1-J 5.0% 7.2% Direct CPA: BAT 1-J 21% 30.1% Diode pumping has a significant impact on system efficiencies, but direct CPA lasers with multi-pulse extraction and cw- pumping will have even greater impact on efficiency and system feasibility for laser-plasma accelerator applications 40

The repetition rate has a significant effect on the extraction and system efficiencies, depending on laser media Example: Yb-fiber Direct CPA Single-Pulse Extraction Multi-Pulse Extraction 92% 1/gain-lifetime 100/gain-lifetime 11% Direct CPA: Low-PRF Direct CPA: High-PRF Waste 1-J Output Efficiency WP EO 26% 34% 1-J 2.0% 2.9% -50-40 -30-20 -10 0 Energy [J per J of short-pulse output] 41

LLNL 3.3 MW solar farm can power ~2x BAT 1 mile 42

Summary We have developed a conceptual design for a single-aperture, 300 kw Thulium:YLF Petawatt-class laser BAT consistent with requirements for laser wakefield accelerators The underlying technology is a modest extension of established LLNL gas-cooling and rep rated Petawatt technologies BAT makes use of a highly simplified laser architecture, multi-pulse extraction of CWdiode pumped Tm:YLF and thus providing good wall-plug-efficiency We have developed a list of system TRLs and challenges that will inform the strategic plan for R&D and RTP efforts System Type TRL Estimate Integration Challenge delivery horizon E (J) t (fs) P av (kw) P peak (PW) HAPLS DPSSL+TiS 7 Low today 30 <30 0.3 1 SHARC DP CPA Nd:Glass 6 Low 3yrs 150 150 1.5 1 Mini-BAT DP CPA Tm:YLF 3-4 Medium 3-5yrs 3 BAT DP CPA Tm:YLF 3 Medium 5-7yrs 30 40 or 100 40 or 100 3.075 300.75 43

Questions? Postdoc? Job? Dr. Constantin Haefner Program Director haefner2@llnl.gov