Herzlich willkommen. Druckbare Sensoren für Food Packaging ICT-Agri-Food Symposium. Sören Fricke Section Head Large Area & Flexible Systems

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1 Herzlich willkommen Druckbare Sensoren für Food Packaging ICT-Agri-Food Symposium Sören Fricke Section Head Large Area & Flexible Systems Agroscope Tänikon,

2 Motivation Printed Sensors can be produced on low-cost substrates e.g. PET Printed Sensors can be produced on bio-degradable materials Printed Sensors and flexible hybrid electronics can be produced on large areas (rolls) Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 1

3 Printing Technologies and Materials Non-contact printing technologies e.g. Ink-jet printing Aerosoljet printing Screen-printing Slot-die Coating Contact printing technologies e.g. Semiconductors Organic, Inorganic (PEDOT, P3HT, Si, ) Dielectrics Organic, Inorganic (PS, PMMA, BCB, Oxides ) Gravure printing Flexography printing Nano-imprinting Conductors Metals (Ag, Cu, Au, Pt,..) Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 2

4 Components, devices, realized by printing Electric discrete components: Wirings, bus bars, electrodes Resistors Inductors Antennas Capacitors Active electronic devices: (Photo-)Diodes Transistors OLEDs Solar cells. Memory devices Ferroelectric capacitors Energy storage Batteries Sensors Physical, chemical Flexible Hybrid Systems Printing + SMD Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 3

5 also printed Sensors build on known sensing principles Capacitive Resistive Inductive Pyroelectric Resonant Optical Amperometric Voltametric Impedance Thermoelectric Piezoresistive Piezoelectric Photoelectric Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 4

6 Physical: Printed Temperature Sensors Inkjet printed Ag RTD on PET (PTC) TCR: C -1 Screen-printed Wheatstone Bridge of NTC (ATO) and PTC materials on PEN F. Molina-Lopez et al V/ 48V in Screen-printed Si nanoparticles (NTC) and Ag electrodes printed on e.g. paper (PST Sensors Ltd.) logarithmic temperature coefficient 2000 ± 100K (T: C) A. Aliane et al. D.T. Britton et al. Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 5

7 Physical: Printed Pressure Sensors Capacitive: CNT-doped PDMS electrodes on PDMS, by soft-lithography and blade coating Piezoresistive: Screen-printing of Ag electrodes and Carbon ink as piezoresistive layer on PU. Woo et al. Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 6

8 Physical: Printed Strain Sensors Piezoresistive: Aerosoljet printed PEDOT:PSS on Kapton substrate Gauge factor 0.53 B. Thompson et al. Piezoresistive: Screen-printing of CNT-AgNP paste on silicone Ratio of CNT in the paste tunes strain sensitivity and temperature insensitivity S. Harada et al. Sensitivity 59%/Pa in linear regime Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 7

9 Physical: Printed Photodetectors Photodiodes: Fully inkjet printed Ag, PEDOT:PSS, P3HT:PCBM Passive Matrix Imager: inkjet printed P3HT:PCBM. 128dpi demonstrated, 512dpi under development G. Azzellino et al. Active Matrix Imager: ISORG building manufacturing site in Limoges (France) ISORG Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 8

10 Chemical: Electrochemical Sensors Electrical Read-out:Voltametry, Amperometry or Impedance-Spectrocsopy Principal: Functionalization with Antibodies Sensing: glucose, ph, lactate, cancer biomarkers.. screen-printed sensors with Ag, C, AgCl, Au, electrodes have reached mass-production G.C. Jensen et al. Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 9

11 Chemical: Printed Ion Sensors cont. a) OFET: Semiconductor exposed OFET b) Ion-sensitive OFET (ISOFET): Insulator exposed OFET c) Organic electrochemical transistor (OECT): Insulator dielectric replaced by electrolyte OECT humidity sensor on PE coated paper using PEDOT:PSS as organic semiconductor and Nafion as electrolyte D. Nilson et al. J.T. Mabeck et al. Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 10

12 Chemical: Printed Gas Sensors Au and Pd decorated carbon-nanofibres on Kapton. Inkjet printed Ag electrodes and heater. Ammonia and NO 2 sensor S. Claramunt et al. Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 11

13 Printed Sensors vs. MEMS Sensors BOSCH Automotive Rigid package, silicone glue, rigid die with SiN membrane and glass socket Cross-sensitivities minimized by thermo-mechnical decoupling Mounting SMD Local measurement PU foil bendable, stetchable Cross-sensitive to bending, stretching, Temperature Mounting on surfaces Mapping Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 12

14 Summary Printed Sensors have been demonstrated with many sensing principles Very different levels of maturity, some are commercialized, some are lab prototypes Strong potential in chemical and biological sensors Integrating communication chips can increase the costs Food packaging of precious goods All large area applications can benefit from the integration on foil by printing Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 13

15 Thank you for your attention!

16 Chemical: Electrochemical Sensors cont. Inkjet printed Au NP electrodes on Kapton cancer biomarker interleukin-6 (IL-6) in serum Gravure-printed Ag NP electrodes on PET G.C. Jensen et al. mercury sulfide (HgS), lead sulfide (PbS), D-proline and sarcosine B.B. Narakathu et al. Copyright 2017 CSEM Gedruckte Sensoren Sören Fricke Page 19

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